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Superconductive hydrogen-rich compounds under high pressure

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Abstract

In recent decades, hydrogen-rich compounds are promising candidates for room-temperature superconductors under extremely high pressure. Remarkably, the theory-oriented finding of covalent hydride H3S and a class of clathrate hydrides, such as YH9 and LaH10, with high superconducting critical temperature (Tc) above 240 K, which give rise to the hope of searching for room-temperature superconductivity among hydrogen-rich compounds under high pressure. In this paper, we focus on the research progress of binary and ternary hydrides, provide the introduction of conventional phonon-mediated superconductivity theory and the physical mechanism of high-temperature superconductivity briefly, and offer an outlook on the challenge of discovering room-temperature superconductors among hydrogen-rich compounds in the future.

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References

  1. H.K. Onnes, The Resistance of Pure Mercury at Helium Temperatures (Springer, Dordrecht, 1911)

    Google Scholar 

  2. Y. Tokura, H. Takagi, S. Uchida, Nature 337, 345–347 (1989)

    Article  ADS  Google Scholar 

  3. W.M. Lia, J.F. Zhao, L.P. Cao, Z. Hud, Q.Z. Huange, X.C. Wang, Y. Liu, G.Q. Zhao, J. Zhang, Q.Q. Liu, R.Z. Yu, Y.W. Long, H. Wu, H.J. Lin, C.T. Chenf, Z. Lig, Z.Z. Gongh, Z. Guguchiah, J.S. Kimi, G.R. Stewarti, Y.J. Uemurah, S. Uchida, C.Q. Jin, Proc. Natl. Acad. Sci. U. S. A. 116, 12156–12160 (2019)

    Article  ADS  Google Scholar 

  4. J. Nagamatsu, N. Nakagawa, T. Muranaka, Y. Zenitani, J. Akimitsu, Nature 410, 63–64 (2001)

    Article  ADS  Google Scholar 

  5. L. Gao, Z.J. Huang, R.L. Meng, J.G. Lin, F. Chen, L. Beauvais, Y.Y. Sun, Y.Y. Xue, C.W. Chu, Phys. C 213, 261–265 (1993)

    Article  ADS  Google Scholar 

  6. J.G. Bednorz, K.A. Müller, Z. Phys. B: Condens. Matter 64, 189–193 (1986)

    Article  ADS  Google Scholar 

  7. M.K. Wu, J.R. Ashburn, C.J. Torng, Phys. Rev. Lett. 58, 908–910 (1987)

    Article  ADS  Google Scholar 

  8. B.W. Statt, Z. Wang, M.J.G. Lee, J.V. Yakhmi, P.C. De Camargo, Phys. C 156, 251–255 (1988)

    Article  ADS  Google Scholar 

  9. M.A. Subramanian, J.C. Calabrese, C.C. Torardi, J. Gopalakrishnan, T.R. Askew, R.B. Flippen, K.J. Morrissey, U. Chowdhry, A.W. Sleight, Nature 332, 420–422 (1988)

    Article  ADS  Google Scholar 

  10. A. Schilling, M. Cantoni, J.D. Guo, H.R. Ott, Nature 363, 56–58 (1993)

    Article  ADS  Google Scholar 

  11. L. Gao, Y.Y. Xue, F. Chen, Q. Xiong, R.L. Meng, D. Ramirez, C.W. Chu, Phys. Rev. B 50, 4260–4263 (1994)

    Article  ADS  Google Scholar 

  12. H. Takahashi, K. Igawa, K. Arii, Y. Kamihara, M. Hirano, H. Hosono, Nature 453, 376–387 (2008)

    Article  ADS  Google Scholar 

  13. Z.A. Ren, W. Lu, J. Yang, W. Yi, X.L. Shen, Z.C. Li, G.C. Che, X.L. Dong, L.L. Sun, F. Zhou, Z.X. Zhao, Chin. Phys. Lett. 25, 2215–2216 (2008)

    Article  ADS  Google Scholar 

  14. J. Bardeen, L.N. Cooper, J.R. Schrieffer, Phys. Rev. 108, 1175–1204 (1956)

    Article  ADS  Google Scholar 

  15. N.W. Ashcroft, Phys. Rev. Lett. 21, 1748–1749 (1968)

    Article  ADS  Google Scholar 

  16. P.D. Simpson, R.T. Howie, E. Gregoryanz, Nature 529, 63–67 (2016)

    Article  ADS  Google Scholar 

  17. R.P. Dias, I.F. Silvera, Science 355, 1–9 (2017)

    Article  Google Scholar 

  18. C.B. Satterthwaite, I.L. Toepke, Phys. Rev. Lett. 25, 741–743 (1970)

    Article  ADS  Google Scholar 

  19. T. Skoskiewicz, Phys. Status Solidi B 59, 329–334 (1973)

    Article  ADS  Google Scholar 

  20. W. Buckel, A. Eichler, B. Stritzker, Z. Phys. A: Hadrons Nucl. 263, 1–4 (1973)

    Article  Google Scholar 

  21. B. Stritzker, Z. Phys. A: Hadrons Nucl. 268, 261–264 (1974)

    Article  Google Scholar 

  22. J.M. Welter, F.J. Johnen, Z. Phys. B: Condens Matter. 27, 227–232 (1977)

    Article  ADS  Google Scholar 

  23. A.E. Carlsson, N.W. Ashcroft, Phys. Rev. Lett. 50, 1305–1308 (1983)

    Article  ADS  Google Scholar 

  24. N.W. Ashcroft, Phys. Rev. Lett. 92, 187002 (2004)

    Article  ADS  Google Scholar 

  25. L.J. Zhang, Y.C. Wang, J. Lv, Y.M. Ma, Nat. Rev. Mater. 2, 1–16 (2017)

    ADS  Google Scholar 

  26. D.F. Duan, Y.X. Liu, Y.B. Ma, Z.J. Shao, B.B. Liu, T. Cui, Natl. Sci. Rev. 4(2017), 121–135 (2017)

    Article  Google Scholar 

  27. Y.C. Wang, Y.M. Ma, J. Chem. Phys. 140, 040901 (2014)

    Article  ADS  Google Scholar 

  28. M.I. Eremets, I.A. Trojan, S.A. Medvedev, J.S. Tes, Y. Yao, Science 319, 1506–1509 (2008)

    Article  ADS  Google Scholar 

  29. H.K. Mao, X.J. Chen, Y. Ding, B. Li, L. Wang, Rev. Mod. Phys. 90, 015007 (2018)

    Article  ADS  Google Scholar 

  30. C. Buzea, K. Robbie, Supercond. Sci. Technol. 18, R1–R8 (2005)

    Article  ADS  Google Scholar 

  31. K. Shimiu, Phys. C 514(2015), 46–49 (2015)

    Article  ADS  Google Scholar 

  32. C.R. Rotundu, T. Cuk, R.L. Greene, Z.X. Shen, R.J. Hemlty, Rev. Sci. Instrum. 84, 063903 (2013)

    Article  ADS  Google Scholar 

  33. Y.C. Wang, J. Lv, L. Zhu, Y.M. Ma, Comput. Phys. Commun. 183, 2063–2070 (2012)

    Article  ADS  Google Scholar 

  34. M. Jansen, Adv. Mater. 27, 3229–3242 (2015)

    Article  Google Scholar 

  35. H.Y. Liu, W.W. Cui, Y.M. Ma, J. Chem. Phys. 137, 184502 (2012)

    Article  ADS  Google Scholar 

  36. E. Zurek, W. Grochala, Phys. Chem. Chem. Phys. 17, 2917–2934 (2015)

    Article  Google Scholar 

  37. A.P. Drozdov, M.I. Eremets, I.A. Troyan, V. Ksenofontov, S.I. Shylin, Nature 525, 73–76 (2015)

    Article  ADS  Google Scholar 

  38. A.P. Drozdov, P.P. Kong, V.S. Minkov, S.P. Besedin, M.A. Kuzovnikov, S. Mozaffari, L. Balicas, F.F. Balakirev, D.E. Graf, V.B. Prakapenka, E. Greenberg, D.A. Knyazev, M. Tkacz, M.I. Eremets, Nature 569, 528–531 (2019)

    Article  ADS  Google Scholar 

  39. M. Somayazulu, M. Ahart, A.K. Mishra, Z.M. Geballe, M. Baldini, Y. Meng, V.V. Struzhkin, R.J. Hemley, Phys. Rev. Lett. 122, 027001 (2019)

    Article  ADS  Google Scholar 

  40. W.L. McMillan, Phys. Rev. 167, 331–344 (1968)

    Article  ADS  Google Scholar 

  41. P.B. Allen, R.C. Dynes, Phys. Rev. B 12, 905–922 (1975)

    Article  ADS  Google Scholar 

  42. R.C. Dynes, Solid State Commun. 10, 615–618 (1972)

    Article  ADS  Google Scholar 

  43. E. Zurek, T. Bi, J. Chem. Phys. 150, 050901 (2019)

    Article  ADS  Google Scholar 

  44. J.A.F. Livas, L. Boeri, A. Sanna, G. Profeta, R. Arita, M. Eremets, Phys. Rep. 856, 1–78 (2020)

    Article  ADS  MathSciNet  Google Scholar 

  45. H. Wang, J.S. Tse, K. Tanaka, T. Iitaka, Y.M. Ma, Proc. Natl. Acad. Sci. U. S. A. 109, 6463–6466 (2012)

    Article  ADS  Google Scholar 

  46. W.H. Chen, D.V. Semenok, A.G. Kvashnin, X.L. Huang, I.A. Kruglov, M. Galasso, H. Song, D.F. Duan, A.F. Goncharov, V.B. Prakapenka, A.R. Oganov, T. Cui, Nat. Commun. 12, 1–9 (2021)

    Article  Google Scholar 

  47. D.V. Semenok, A.G. Kvashnin, I.A. Kruglov, A.R. Oganov, J. Phys. Chem. Lett. 9, 1920–1926 (2018)

    Article  Google Scholar 

  48. S.F. Qian, X.W. Sheng, X.Z. Yan, Y.M. Chen, B. Song, Phys. Rev. B 96, 094513 (2017)

    Article  ADS  Google Scholar 

  49. X.L. Feng, J.R. Zhang, G.Y. Gao, H.Y. Liu, H. Wang, RSC Adv. 5, 1–3 (2015)

    Article  Google Scholar 

  50. T.A. Strobel, P. Ganesh, M. Somayazulu, P.R.C. Kent, R.J. Hemley, Phys. Rev. Lett. 107, 255503 (2011)

    Article  ADS  Google Scholar 

  51. J. Lv, Y. Sun, H.Y. Liu, Y.M. Ma, Matter Radiat. Extremes 5, 068101 (2020)

    Article  Google Scholar 

  52. Y. Sun, H.Y. Liu, Y.M. Ma, Acta Phys. Sin. 70, 017407 (2021)

    Article  Google Scholar 

  53. H.F. Li, X. Li, H. Wang, G.T. Liu, Y.W. Li, H.Y. Liu, New J. Phys. 21, 123009 (2019)

    Article  Google Scholar 

  54. Y.W. Li, J. Hao, H.Y. Liu, Y.L. Li, Y.M. Ma, J. Chem. Phys. 140, 174712 (2014)

    Article  ADS  Google Scholar 

  55. D.F. Duan, Y.X. Liu, F.B. Tian, D. Li, X.L. Huang, Z.L. Zhao, H.Y. Yu, B.B. Liu, W.J. Tian, T. Cui, Sci. Rep. 4, 6989 (2014)

    Article  Google Scholar 

  56. Y.S. Yao, J.S. Tse, Chem. Eur. J. 24, 1–25 (2017)

    Google Scholar 

  57. M. Einaga, M. Sakata, T. Ishikawa, Nat. Phys. 12, 835–838 (2016)

    Article  Google Scholar 

  58. X.L. Huang, X. Wang, D.F. Duan, Nal. Sci. Rev. 6, 713–718 (2019)

    Google Scholar 

  59. A.F. Goncharov, S.S. Lobanov, I. Kruglov, X.M. Zhao, X.J. Chen, A.R. Oganov, Z. Konopkova, V.B. Prakapenka, Phys. Rev. B 93, 174105 (2016)

    Article  ADS  Google Scholar 

  60. B. Guigue, A. Marizy, P. Loubeyre, Phys. Rev. B 95, R020104 (2017)

    Article  ADS  Google Scholar 

  61. F. Alexander, S.S. Goncharov, V.B. Lobanov, Phys. Rev. B 95, R140101 (2017)

    Article  Google Scholar 

  62. E.E. Gordon, K. Xu, H.J. Xiang, A.B. Holder, R.K. Kremer, A. Simon, J. Kçhler, M.H. Whangbo, Angew. Chem. Int. Ed. 55, 3682–3685 (2016)

    Article  Google Scholar 

  63. R. Martonak, A. Laio, M. Parrinello, Phys. Rev. Lett. 90, 075503 (2003)

    Article  ADS  Google Scholar 

  64. A. Majumdar, J.S. Tse, Y.S. Yao, Angew. Chem. Int. Ed. 56, 11390–11393 (2017)

    Article  Google Scholar 

  65. A. Majumdar, J.S. Tse, Y.S. Yao, Sci. Rep. 9, 5023 (2019)

    Article  ADS  Google Scholar 

  66. W.D. Zhao, D.F. Duan, T. Cui, Chin. J. High Press. Phys. 35, 020101 (2021)

    Google Scholar 

  67. K. Tanaka, J.S. Tse, H. Liu, Phys. Rev. B 96, 100502 (2017)

    Article  ADS  Google Scholar 

  68. I. Errea, M. Calandra, C.J. Pickard, J.R. Nelson, R.J. Needs, Y.W. Li, H.Y. Liu, Y.W. Zhang, Y.M. Ma, F. Mauri, Nature 532, 81–84 (2016)

    Article  ADS  Google Scholar 

  69. F. Peng, Y. Sun, C.J. Pickard, R.J. Needs, Q. Wu, Y.M. Ma, Phys. Rev. Lett. 119, 107001 (2017)

    Article  ADS  Google Scholar 

  70. N.P. Salke, M. Mahdi, D. Esfahani, Y.J. Zhang, I.A. Kruglov, J.S. Zhou, Y.G. Wang, E. Greenberg, V.B. Prakapenka, J. Liu, A.R. Oganov, J.F. Lin, Nat. Commun. 10, 1–10 (2019)

    Article  Google Scholar 

  71. D.V. Semenok, D. Zhou, A.G. Kvashnin, X.L. Huang, M. Galasso, I.A. Kruglov, A.G. Ivanova, A.G. Gavriliuk, W.H. Chen, N.V. Tkachenko, A.I. Boldyrev, I. Troyan, A.R. Oganov, T. Cui, J. Phys. Chem. 12, 32–40 (2021)

    Google Scholar 

  72. X. Li, X.L. Huang, D.F. Duan, C.J. Pickard, D. Zhou, H. Xie, Q. Zhuang, Y.P. Huang, Q. Zhou, B.B. Liu, T. Cui, Nat. Commun. 10, 1–7 (2019)

    Article  ADS  Google Scholar 

  73. D.V. Semenok, A.G. Kvashnin, A.G. Ivanova, V. Svitlyk, V.Y. Fominski, A.V. Sadakov, O.A. Sobolevskiy, V.M. Pudalov, I.A. Troyan, A.R. Ogano, Mater. Today 33, 36–44 (2019)

    Article  Google Scholar 

  74. X.Q. Ye, N. Zarifi, E. Zurek, R. Hoffmann, N.W. Ashcroft, J. Phys. Chem. C 122, 6298–6309 (2018)

    Article  Google Scholar 

  75. H.Y. Liu, I.I. Naumov, R. Hoffmann, N.W. Ashcroft, R.J. Hemley, Proc. Natl. Acad. Sci. U. S. A. 114, 6990–6995 (2017)

    Article  ADS  Google Scholar 

  76. W.G. Sun, X.Y. Kuang, H.D.J. Keen, C. Lu, A. Hermann, Phys. Rev. B 102, 144524 (2020)

    Article  ADS  Google Scholar 

  77. H.Y. Liu, I. Naumov, Z.M. Geballe, M. Somayazulu, J.S. Tse, R.J. Hemley, Phys. Rev. B 98, R100102 (2018)

    Article  ADS  Google Scholar 

  78. P. P. Kong, V. S. Minkov, M. A. Kuzovnikov, S. P. Besedin, A. P. Drozdov, S. Mozaffari, L. Balicas, F. F. Balakirev, V. B. Prakapenka, E. Greenberg, D. A. Knyazev, M. I. Eremets, arXiv 1909 10482

  79. I.A. Troyan, D.V. Semenok, A.G. Kvashnin, A.V. Sadakov, O.A. Sobolevskiy, V.M. Pudalov, A.G. Ivanova, V.B. Prakapenka, E. Greenberg, A.G. Gavriliuk, I.S. Lyubutin, V.V. Struzhkin, A. Bergara, I. Errea, R. Bianco, M. Calandra, F. Mauri, L. Monacelli, R. Akashi, A.R. Oganov, Adv. Mater. 33, 2006832 (2021)

    Article  Google Scholar 

  80. C.M. Pépin, G. Geneste, A. Dewaele, M. Mezouar, Science 357, 382–385 (2017)

    Article  ADS  Google Scholar 

  81. X. Zhong, H. Wang, J.R. Zhang, H.Y. Liu, S.T. Zhang, H.F. Song, G.C. Yang, L.J. Zhang, Y.M. Ma, Phys. Rev. Lett. 116, 057002 (2016)

    Article  ADS  Google Scholar 

  82. D.W. Zhou, X.L. Jin, X. Meng, G. Bao, Y.M. Ma, B.B. Liu, T. Cui, Phys. Rev. B 86, 014118 (2012)

    Article  ADS  Google Scholar 

  83. H. Xie, Y.S. Yao, X.L. Feng, D.F. Duan, H. Song, Z.H. Zhang, S.Q. Jiang, S.A.T. Redfern, V.Z. Kresin, C.J. Pickard, T. Cui, Phys. Rev. Lett. 125, 217001 (2020)

    Article  ADS  Google Scholar 

  84. T. G. Bi, N. Zarifi, T. Terpstra, E. Zurek, arXiv: 1806.00163

  85. Y. Sun, J. Lv, Y. Xie, H.Y. Liu, Y.M. Ma, Phys. Rev. Lett. 123, 097001 (2019)

    Article  ADS  Google Scholar 

  86. H. Wang, Y.S. Yao, F. Peng, H.Y. Liu, R.J. Hemley, Phys. Rev. Lett. 126, 117002 (2021)

    Article  ADS  Google Scholar 

  87. X.W. Liang, A. Bergara, L.Y. Wang, B. Wen, Z.S. Zhao, X.F. Zhou, J.L. He, G.Y. Gao, Y.J. Tian, Phys. Rev. B 99, 100505 (2019)

    Article  ADS  Google Scholar 

  88. E. Snider, N.D. Gammon, R. McBride, M. Debessai, H. Vindana, K. Vencatasamy, K.V. Lawler, A. Salamat, R.P. Dias, Nature 586, 373–377 (2020)

    Article  ADS  Google Scholar 

  89. A. D. Grockowiak, M. Ahart, T. Helm, W. A. Coniglio, R. Kumar, M. Somayazulu, Y. Meng, M. Oliff, V. Williams, N. W. Ashcroft, R. J. Hemley, S. W. Tozer, arXiv: 2006.03004

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Acknowledgements

This research was supported by the Natural Science Foundation of China (grant no. 11504007 and 12074138) and the Scientific and Technological Research Project of the “13th Five-Year Plan” of Jilin Provincial Education Department (grant no. JJKH20200031KJ).

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Zhang, S., Zhang, M. & Liu, H. Superconductive hydrogen-rich compounds under high pressure. Appl. Phys. A 127, 684 (2021). https://doi.org/10.1007/s00339-021-04802-4

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