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Existence of a magnetically ordered hole gas at the La0.7Sr0.3MnO3/SrRuO3 interface

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Abstract

The study of spatially confined complex oxides is of wide interest, since correlated electrons at interfaces might form new states of matter. Here La0.7Sr0.3MnO3/SrRuO3 superlattices with coherently grown interfaces and layer thicknesses down to one unit cell were fabricated by pulsed laser deposition. The superlattices were studied by X-ray, HRTEM, magnetization and magnetotransport measurements. For such small thicknesses La0.7Sr0.3MnO3 films are antiferromagnetic and insulating. Despite the small layer thickness, the LaSrMnO layers in the superlattices were ferromagnetic with Curie temperatures close to room temperature. Whereas the resistivity of the superlattices showed metallic behaviour and was dominated by the conducting SrRuO3 layers, the off-diagonal resistivity showed an anomalous Hall effect with ferromagnetic loop shape even far above the Curie temperature of the SrRuO3 layers as well as a positive high field slope. This indicates the presence of a highly conducting, ferromagnetically ordered hole gas at the interfaces that might be formed by a charge-transfer process. This result opens up an alternative route for the fabrication of quasi-two-dimensional systems.

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References

  1. M. Bibes, J.E. Villegas, A. Barthélémy, Adv. Phys. 60, 5 (2011)

    Article  ADS  Google Scholar 

  2. V. Garcia, M. Bibes, L. Bocher, S. Valencia, F. Kronast, A. Crassous, X. Moya, S. Enouz-Vedrenne, A. Gloter, D. Imhoff, C. Deranlot, N.D. Mathur, S. Fusil, K. Bouzehouane, A. Barthélémy, Science 327, 1106 (2010)

    Article  ADS  Google Scholar 

  3. J. Mannhart, D.G. Schlom, Science 327, 1607 (2010)

    Article  ADS  Google Scholar 

  4. S.A. Chambers, M.H. Engelhard, V. Shutthanandan, Z. Zhu, T.C. Droubay, L. Qiao, P.V. Sushko, T. Feng, H.D. Lee, T. Gustafsson, E. Garfunkel, A.B. Shah, J.-M. Zuo, Q.M. Ramasse, Surf. Sci. Rep. 65, 317 (2010)

    Article  ADS  Google Scholar 

  5. Ariando, X. Wang, G. Baskaran, Z.Q. Liu, J. Huijben, J.B. Yi, A. Annadi, A.R. Barman, A. Rusydi, S. Dhar, Y.P. Feng, J. Ding, H. Hilgenkamp, T. Venkatesan, Nature Commun. 2, 188 (2011)

    Article  ADS  Google Scholar 

  6. D.A. Dikin, M. Mehta, C.W. Bark, C.M. Folkman, C.B. Eom, V. Chandrasekhar, Phys. Rev. Lett. 107, 056802 (2011)

    Article  ADS  Google Scholar 

  7. Y. Konishi, Z. Fang, M. Izumi, T. Manako, M. Kasai, H. Kuwahara, M. Kawasaki, K. Terakura, Y. Tokura, J. Phys. Soc. Jpn 68, 3790 (1999)

    Article  ADS  Google Scholar 

  8. Z. Fang, I.V. Solovyev, K. Terakura, Phys. Rev. Lett. 84, 3169 (2000)

    Article  ADS  Google Scholar 

  9. M. Ziese, H.C. Semmelhack, K.-H. Han, Phys. Rev. B 68, 134444 (2003)

    Article  ADS  Google Scholar 

  10. M. Huijben, L.W. Martin, Y.-H. Chu, M.B. Holcomb, P. Yu, G. Rijnders, D.H.A. Blank, R. Ramesh, Phys. Rev. B 78, 094413 (2008)

    Article  ADS  Google Scholar 

  11. A. Tebano, C. Aruta, S. Sanna, P.G. Medaglia, G. Balestrino, A.A. Sidorenko, R. De Renzi, G. Ghiringhelli, L. Braicovich, V. Bisogni, N.B. Brookes, Phys. Rev. Lett. 100, 137401 (2008)

    Article  ADS  Google Scholar 

  12. A. Baena, L. Brey, M.J. Calderón, Phys. Rev. B 83, 064424 (2011)

    Article  ADS  Google Scholar 

  13. Moon-Ho Jo, N.D. Mathur, N.K. Todd, M.G. Blamire, Phys. Rev. B 61, R14905 (2000)

    Article  ADS  Google Scholar 

  14. M. Bibes, Ll. Balcells, S. Valencia, J. Fontcuberta, M. Wojcik, E. Jedryka, S. Nadolski, Phys. Rev. Lett. 87, 067210 (2001)

    Article  ADS  Google Scholar 

  15. H. Yamada, Y. Ogawa, Y. Ishii, H. Sato, M. Kawasaki, H. Akoh, Y. Tokura, Science 305, 646 (2004)

    Article  ADS  Google Scholar 

  16. X. Ke, M.S. Rzchowski, L.J. Belenky, C.B. Eom, Appl. Phys. Lett. 84, 5458 (2004)

    Article  ADS  Google Scholar 

  17. X. Ke, L.J. Belenky, C.B. Eom, M.S. Rzchowski, J. Appl. Phys. 97, 10K115 (2005)

    Article  Google Scholar 

  18. P. Padhan, W. Prellier, R.C. Budhani, Appl. Phys. Lett. 88, 192509 (2006)

    Article  ADS  Google Scholar 

  19. M. Ziese, I. Vrejoiu, E. Pippel, P. Esquinazi, D. Hesse, C. Etz, J. Henk, A. Ernst, I.V. Maznichenko, W. Hergert, I. Mertig, Phys. Rev. Lett. 104, 167203 (2010)

    Article  ADS  Google Scholar 

  20. Y. Lee, B. Caes, B.N. Harmon, J. Alloys Comp. 450, 1 (2008)

    Article  Google Scholar 

  21. J.X. Ma, X.F. Liu, T. Lin, G.Y. Gao, J.P. Zhang, W.B. Wu, X.G. Li, Jing Shi, Phys. Rev. B 79, 174424 (2009)

    Article  ADS  Google Scholar 

  22. M.C. Dekker, A. Herklotz, L. Schultz, M. Reibold, K. Vogel, M.D. Biegalski, H.M. Christen, K. Dörr, Phys. Rev. B 84, 054463 (2011)

    Article  ADS  Google Scholar 

  23. R. Hillebrand, E. Pippel, D. Hesse, I. Vrejoiu, Phys. Status Solidi A 208, 2144 (2011)

    Article  ADS  Google Scholar 

  24. M.E. Fisher, M.N. Barber, Phys. Rev. Lett. 28, 1516 (1972)

    Article  ADS  Google Scholar 

  25. Y.J. Chang, C.H. Kim, S.-H. Phark, Y.S. Kim, J. Yu, T.W. Noh, Phys. Rev. Lett. 103, 057201 (2009)

    Article  ADS  Google Scholar 

  26. M. Izumi, K. Nakazawa, Y. Bando, J. Phys. Soc. Jpn 67, 651 (1998)

    Article  ADS  Google Scholar 

  27. L. Fitting Kourkoutis, J.H. Song, H.Y. Hwang, D.A. Muller, Proc. Natl. Acad. Sci. 107, 11682 (2010)

    Article  ADS  Google Scholar 

  28. H. Yamada, M. Kawasaki, Y. Tokura, Appl. Phys. Lett. 86, 192505 (2005)

    Article  ADS  Google Scholar 

  29. S. Brivio, C. Magen, A.A. Sidorenko, D. Petti, M. Cantoni, M. Finazzi, F. Ciccacci, R. De Renzi, M. Varela, S. Picozzi, R. Bertacco, Phys. Rev. B 81, 094410 (2010)

    Article  ADS  Google Scholar 

  30. M. Ziese, I. Vrejoiu, D. Hesse, Phys. Rev. B 81, 184418 (2010)

    Article  ADS  Google Scholar 

  31. M. Ziese, I. Vrejoiu, D. Hesse, Appl. Phys. Lett. 97, 052504 (2010)

    Article  ADS  Google Scholar 

  32. N. Nagaosa, J. Sinova, S. Onoda, A.H. MacDonald, N.P. Ong, Rev. Mod. Phys. 82, 1539 (2010)

    Article  ADS  Google Scholar 

  33. G. Jakob, F. Martin, W. Westerburg, H. Adrian, Phys. Rev. B 57, 10252 (1998)

    Article  ADS  Google Scholar 

  34. M. Ziese, C. Srinitiwarawong, Europhys. Lett. 45, 256 (1999)

    Article  ADS  Google Scholar 

  35. P. Matl, N.P. Ong, Y.F. Yan, Y.Q. Li, D. Studebaker, T. Baum, G. Doubinina, Phys. Rev. B 57, 10248 (1998)

    Article  ADS  Google Scholar 

  36. R. Mathieu, A. Asamitsu, H. Yamada, K.S. Takahashi, M. Kawasaki, Z. Fang, N. Nagaosa, Y. Tokura, Phys. Rev. Lett. 93, 016602 (2004)

    Article  ADS  Google Scholar 

  37. M. Ziese, I. Vrejoiu, Phys. Rev. B 84, 104413 (2011)

    Article  ADS  Google Scholar 

  38. M. Ziese, F. Bern, E. Pippel, D. Hesse, I. Vrejoiu, Nanophys. Lett. 12, 4276 (2012)

    Article  Google Scholar 

  39. Y. Kats, I. Genish, L. Klein, J.W. Reiner, M.R. Beasley, Phys. Rev. B 70, 180407(R) (2004)

    ADS  Google Scholar 

  40. B.R.K. Nanda, S. Satpathy, M.S. Springborg, Phys. Rev. Lett. 98, 216804 (2007)

    Article  ADS  Google Scholar 

  41. J.W. Freeland, J. Chakhalian, A.V. Boris, J.-M. Tonnerre, J.J. Kavich, P. Yordanov, S. Grenier, P. Zschack, E. Karapetrova, P. Popovich, H.N. Lee, B. Keimer, Phys. Rev. B 81, 094414 (2010)

    Article  ADS  Google Scholar 

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Authors and Affiliations

  1. Division of Superconductivity and Magnetism, University of Leipzig, Leipzig, 04103, Germany

    Michael Ziese, Francis Bern & Annette Setzer

  2. Max Planck Institute of Microstructure Physics, Halle, 06120, Germany

    Eckhard Pippel, Dietrich Hesse & Ionela Vrejoiu

  3. Max Planck Institute for Solid State Research, Stuttgart, 70569, Germany

    Ionela Vrejoiu

Authors
  1. Michael Ziese
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  2. Francis Bern
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  3. Annette Setzer
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  4. Eckhard Pippel
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  5. Dietrich Hesse
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  6. Ionela Vrejoiu
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Correspondence to Michael Ziese.

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Ziese, M., Bern, F., Setzer, A. et al. Existence of a magnetically ordered hole gas at the La0.7Sr0.3MnO3/SrRuO3 interface. Eur. Phys. J. B 86, 42 (2013). https://doi.org/10.1140/epjb/e2012-30646-4

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  • DOI: https://doi.org/10.1140/epjb/e2012-30646-4

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