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Phase evolution, microstructure, thermal stability of (K0.45Na0.45Li0.04La0.02)NbO3–Bi(Ni0.5Zr0.5)O3 ceramics

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Abstract

(K0.45Na0.45Li0.04La0.02)NbO3–Bi(Ni0.5Zr0.5)O3[(1 − x)KNLLN-xBNZ, 0 ≤ x ≤ 0.02] ceramics were fabricated via a traditional solid state reaction method. The addition of BNZ can enhance the electrical properties of KNLLN ceramics. As x = 0.015, the sample had good performance with high εr ~ 1665 and excellent thermal stability (Δε/ε100°C ≤ ± 12%) from 100 to 447 °C, indicating that this ceramic has potential application prospects in wider working-temperature range. The electrical behavior at high temperatures of (1 − x)KNLLN-xBNZ ceramics was also analyzed. The results show that the relaxation induced by the double ionized oxygen vacancies is thermally activated.

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Acknowledgements

This work was supported by the Natural Science Foundation of China (Nos. 11664008 and 61761015), Natural Science Foundation of Guangxi (Nos. 2018GXNSFFA050001, 2017GXNSFDA198027 and 2017GXNSFFA198011).

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Authors and Affiliations

  1. Collaborative Innovation Center for Exploration of Hidden Nonferrous Metal Deposits and Development of New Materials in Guangxi, Key Laboratory of Nonferrous Materials and New Processing Technology, Ministry of Education, School of Materials Science and Engineering, Guilin University of Technology, Guilin, 541004, China

    Xiuli Chen, Jie Sun, Xu Li, Xiao Yan, Xiaoxia Li, Junpeng Shi, Congcong Sun, Feihong Pang & Huanfu Zhou

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  1. Xiuli Chen
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  2. Jie Sun
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  3. Xu Li
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Correspondence to Xiuli Chen.

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Chen, X., Sun, J., Li, X. et al. Phase evolution, microstructure, thermal stability of (K0.45Na0.45Li0.04La0.02)NbO3–Bi(Ni0.5Zr0.5)O3 ceramics. J Mater Sci: Mater Electron 30, 16407–16414 (2019). https://doi.org/10.1007/s10854-019-02014-4

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