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Multiphoton absorption of broad-band CO2 laser radiation by SF6

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Abstract

Increase of the emission bandwidth of a high-pressure CO2 laser up to 1.5 cm−1 increases the multiphoton absorption cross-section of SF6. Comparison with the previously found [9] increased absorption for shorter pulses suggests that this is also a bandwidth effect. Spectral structures as narrow as 1 cm−1 above the 10th absorption step are invoked to explain the observations. The temperature effect, which disappears in the broad-band case, confirms this view.

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References

  1. W. Fuß, K.L. Kompa: Prog. Quant. Electr.7, 117 (1981)

    Google Scholar 

  2. S.S. Alimpiev, S.I. Valyanskiy, S.M. Nikiforov, V.V. Smirnov, B.G. Sartakov, V.I. Fabelinskiy, A.L. Shtarkov: JETP Lett.35, 361 (1982)

    Google Scholar 

  3. D.P. Hodgkinson, A.J. Taylor, D.W. Wright, A.G. Robiette: Chem. Phys. Lett.90, 230 (1982); J. Phys. B14, 1803 (1981)

    Google Scholar 

  4. A.J. Taylor, D.P. Hodgkinson, A.G. Robiette: Opt. Commun.41, 320 (1982)

    Google Scholar 

  5. C.W. Patterson, B.J. Krohn, A.S. Pine: Opt. Lett.6, 39 (1981)

    Google Scholar 

  6. C. Di Lauro, F. Lattanzi: Chem. Phys.71, 233 (1982)

    Google Scholar 

  7. C. Di Lauro, F. Lattanzi, G. Sanna: Chem. Phys.73, 215 (1982)

    Google Scholar 

  8. J.G. Black: Thesis, Harvard University (1980)

  9. J.G. Black, P. Kolodner, M.J. Schultz, E. Yablonovitch, N. Bloembergen: Phys. Rev. A19, 704 (1979)

    Google Scholar 

  10. H.S. Kwok, E. Yablonovitch, N. Bloembergen: Phys. Rev. A23, 3094 (1981)

    Google Scholar 

  11. W. Fuß: Chem. Phys.76, 343 (1983)

    Google Scholar 

  12. Wan Chong-yi, C. Schwab, W. Fuß, K.L. Kompa: Opt. Commun46, 311 (1983)

    Google Scholar 

  13. P. Kolodner, H.S. Kwok, J.G. Black, E. Yablonovitch: Opt. Lett.4, 38 (1979)

    Google Scholar 

  14. M.O. Bulanin, I.A. Popov: Sov. Techn. Phys. Lett.4, 557 (1978)

    Google Scholar 

  15. P. Vernard, P. Galarneau, S.L. Chin: Opt. Lett.6, 139 (1981)

    Google Scholar 

  16. A.V. Nowak, D.O. Ham: Opt. Lett.6, 185 (1981)

    Google Scholar 

  17. J.R. Ackerhalt, D.O. Ham, A.V. Nowak, C.R. Phipps, S.J. Thomas: IEEE J. QE-19, 1120 (1983)

    Google Scholar 

  18. K. Kim, R.S. McDowell, W.T. King: J. Chem. Phys.73, 36 (1980)

    Google Scholar 

  19. Yu.R. Kolomiiskii, V.S. Marchuk, E.A. Ryabov: Sov. J. Quant. Electr.12, 1139 (1982)

    Google Scholar 

  20. R.V. Ambartzumian, G.N. Makarov, A.A. Puretzky: Opt. Commun.34, 81 (1980)

    Google Scholar 

  21. J.L. Lyman, R.G. Anderson, R.A. Fisher, J.B. Feldman: Opt. Lett.3, 238 (1978); Chem. Phys.45, 325 (1980)

    Google Scholar 

  22. V.M. Apatin, G.N. Makarov: Appl. Phys. B28, 367 (1982); ZhETF84, 15 (1983)

    Google Scholar 

  23. Wei-shin Tsay, C. Riley, D.O. Ham: J. Chem. Phys.70, 3558 (1979)

    Google Scholar 

  24. S.S. Alimpiev, B.O. Zikrin, L. Holz, S.M. Nikiforov, V.V. Smirnov, B.G. Sartakov, V.I. Fabelinskii, A.L. Shtarkov: InLaser Spectroscopy VI, ed. by H.P. Weber and W. Lüthy, Springer Ser. Opt. Sci.40 (Springer, Berlin, Heidelberg, New York 1983) p. 336; ZhETF Pis'ma38, 349 (1983)

    Google Scholar 

  25. W. Fuß: Chem. Phys. Lett.71, 77 (1980)

    Google Scholar 

  26. G. Hancock, A.J. Macrobert: Chem. Phys. Lett.101, 312 (1983)

    Google Scholar 

  27. V.M. Apatin, G.N. Makarov: Appl. Phys. B30, 207 (1983)

    Google Scholar 

  28. R.V. Ambartzumian, G.N. Makarov, A.A. Puretzky: Opt. Commun.34, 81 (1980)

    Google Scholar 

  29. S.D. Smith, W.E. Schmid, F.M.G. Tablas, K.L. Kompa: InLaser Induced Processes in Molecules, ed. by K.L. Kompa, S.D. Smith, Springer Ser. Chem. Phys.6 (Springer, Berlin, Heidelberg, New York 1979)

    Google Scholar 

  30. D.S. King: Adv. Chem. Phys.50, 105 (1982)

    Google Scholar 

  31. M. Quack: Adv. Chem. Phys.50, 395 (1982)

    Google Scholar 

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Alimpiev, S.S., Fuß, W., Kompa, K.L. et al. Multiphoton absorption of broad-band CO2 laser radiation by SF6 . Appl. Phys. B 35, 1–5 (1984). https://doi.org/10.1007/BF00697513

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