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Lifetimes of electronic excitations in unoccupied surface states and the image potential states on Pd(110)

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Abstract

The contribution of inelastic electron-electron scattering to the decay rate of excitations in the surface states and first two image potential states at the Ȳ point on the surface is calculated in the GW approximation, and the quasi-momentum dependence of the corresponding contribution for the surface states is analyzed. The mechanisms of electron scattering in these states are studied, and the temperature dependence of the excitation lifetime is analyzed with allowance for the contribution of the electron-phonon interaction calculated earlier.

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References

  1. E. Knoesel, A. Hotzel, and M. Wolf, Phys. Rev. B: Condens. Matter 57, 12812 (1998).

    Article  ADS  Google Scholar 

  2. M. Aeschlimann, M. Bauer, S. Pawlik, W. Weber, R. Burgermeister, D. Oberli, and H. C. Siegmann, Phys. Rev. Lett. 79, 5158 (1997).

    Article  ADS  Google Scholar 

  3. H. Petek, H. Nagano, and S. Ogawa, Phys. Rev. Lett. 83, 832 (1999).

    Article  ADS  Google Scholar 

  4. I. Campillo, V. M. Silkin, J. M. Pitarke, E. V. Chulkov, A. Rubio, and P. M. Echenique, Phys. Rev. B: Condens. Matter 61, 13484 (2000).

    Article  ADS  Google Scholar 

  5. V. P. Zhukov, F. Aryasetiawan, E. V. Chulkov, and P. M. Echenique, Phys. Rev. B: Condens. Matter 65, 115116 (2002).

    Article  ADS  Google Scholar 

  6. V. P. Zhukov, E. V. Chulkov, and P. M. Echenique, Phys. Rev. Lett. 93, 096401 (2004).

    Article  ADS  Google Scholar 

  7. U. Höfer, I. L. Shumay, Ch. Reuβ, U. Thomann, W. Wallauer, and Th. Fauster, Science (Washington) 277, 1480 (1997).

    Article  Google Scholar 

  8. M. Wolf, E. Knoesel, and T. Hertel, Phys. Rev. B: Condens. Matter 54, 5295(R) (1996).

    Article  ADS  Google Scholar 

  9. E. V. Chulkov, V. M. Silkin, and M. Machado, Surf. Sci. 482-485, 693 (2001).

    Article  ADS  Google Scholar 

  10. S. Link, H. A. Dürr, G. Bihlmayer, S. Blügel, W. Eberhardt, E. V. Chulkov, V. M. Silkin, and P. M. Echenique, Phys. Rev. B: Condens. Matter 63, 115420 (2001).

    Article  ADS  Google Scholar 

  11. H. Petek and S. Ogawa, Annu. Rev. Phys. Chem. 53, 507 (2002).

    Article  ADS  Google Scholar 

  12. A. Schäfer, I. L. Shumay, M. Wiets, M. Weinelt, Th. Fauster, E. V. Chulkov, V. M. Silkin, and P. M. Echenique, Phys. Rev. B: Condens. Matter 61, 13159 (2000).

    Article  ADS  Google Scholar 

  13. M. Weinelt, J. Phys.: Condens. Matter 14, R1099 (2002).

    Article  ADS  Google Scholar 

  14. U. Bovensiepen, Prog. Surf. Sci. 78, 87 (2005).

    Article  ADS  Google Scholar 

  15. A. B. Schmidt, M. Pickel, M. Donath, P. Buczek, A. Ernst, V. P. Zhukov, P. M. Echenique, L. M. Sandratskii, E. V. Chulkov, and M. Weinelt, Phys. Rev. Lett. 105, 197401 (2010).

    Article  ADS  Google Scholar 

  16. R. Díez Muiño, D. Sánchez-Portal, V. M. Silkin, E. V. Chulkov, and P. M. Echenique, Proc. Natl. Acad. Sci. USA 108, 971 (2011).

    Article  ADS  Google Scholar 

  17. E. V. Chulkov, J. Kliewer, R. Berndt, V. M. Silkin, B. Hellsing, S. Crampin, and P. M. Echenique, Phys. Rev. B: Condens. Matter 68, 195422 (2003).

    Article  ADS  Google Scholar 

  18. C. Corriol, V. M. Silkin, D. Sánchez-Portal, A. Arnau, E. V. Chulkov, P. M. Echenique, T. von Hofe, J. Kliewer, J. Kröger, and R. Berndt, Phys. Rev. Lett. 95, 176802 (2005).

    Article  ADS  Google Scholar 

  19. C. H. Schwalb, S. Sachs, M. Marks, A. Schöll, F. Reinert, E. Umbach, and U. Höfer, Phys. Rev. Lett. 101, 146801 (2008).

    Article  ADS  Google Scholar 

  20. P. S. Kirchmann, L. Rettig, X. Zubizarreta, V. M. Silkin, E. V. Chulkov, and U. Bovensiepen, Nat. Phys. 6, 782 (2010).

    Article  Google Scholar 

  21. S. Mathias, A. Ruffing, F. Deicke, M. Wiesenmayer, M. Aeschlimann, and M. Bauer, Phys. Rev. B: Condens. Matter 81, 155429 (2010).

    Article  ADS  Google Scholar 

  22. M. Bauer, S. Pawlik, and M. Aeschlimann, Phys. Rev. B: Condens. Matter 60, 5016 (1999).

    Article  ADS  Google Scholar 

  23. S. Ogawa, H. Nagano, and H. Petek, Phys. Rev. Lett. 82, 1931 (1999).

    Article  ADS  Google Scholar 

  24. A. G. Borisov, J. P. Gauyacq, E. V. Chulkov, V. M. Silkin, and P. M. Echenique, Phys. Rev. B: Condens. Matter 65, 235434 (2002).

    Article  ADS  Google Scholar 

  25. A. G. Borisov, V. Sametoglu, A. Winkelmann, A. Kubo, N. Pontius, J. Zhao, V. M. Silkin, J. P. Gauyacq, E. V. Chulkov, P. M. Echenique, and H. Petek, Phys. Rev. Lett. 101, 266801 (2008).

    Article  ADS  Google Scholar 

  26. S. Achilli, M. I. Trioni, E. V. Chulkov, P. M. Echenique, V. Sametoglu, N. Pontius, A. Winkelmann, A. Kubo, J. Zhao, and H. Petek, Phys. Rev. B: Condens. Matter 80, 245419 (2009).

    Article  ADS  Google Scholar 

  27. A. G. Borisov, T. Hakala, M. J. Puska, V. M. Silkin, N. Zabala, E. V. Chulkov, and P. M. Echenique, Phys. Rev. B: Condens. Matter 76, 121402(R) (2007).

    Article  ADS  Google Scholar 

  28. C. Tournier-Colletta, B. Kierren, Y. Fagot-Revurat, and D. Malterre, Phys. Rev. Lett. 104, 016802 (2010).

    Article  ADS  Google Scholar 

  29. M. Bonn, S. Funk, Ch. Hess, D. N. Denzler, C. Stampfl, M. Scheffler, M. Wolf, and G. Ertl, Science (Washington) 285, 1042 (1999).

    Article  Google Scholar 

  30. H. Nienhaus, Surf. Sci. Rep. 45, 1 (2002).

    Article  ADS  Google Scholar 

  31. C. D. Lindstrom and X.-Y. Zhu, Chem. Rev. (Washington) 106, 4281 (2006).

    Article  Google Scholar 

  32. N. Memmel and E. Bertel, Phys. Rev. Lett. 75, 485 (1995).

    Article  ADS  Google Scholar 

  33. P. M. Echenique, R. Berndt, E. V. Chulkov, Th. Fauster, A. Goldmann, and U. Höfer, Surf. Sci. Rep. 52, 219 (2004).

    Article  Google Scholar 

  34. E. V. Chulkov, A. G. Borisov, J. P. Gauyacq, D. Sánchez-Portal, V. M. Silkin, V. P. Zhukov, and P. M. Echenique, Chem. Rev. (Washington) 106, 4160 (2006).

    Article  Google Scholar 

  35. A. Eiguren, B. Hellsing, E. V. Chulkov, and P. M. Echenique, Phys. Rev. B: Condens. Matter 67, 235423 (2003).

    Article  ADS  Google Scholar 

  36. M. Fuglsang Jensen, T. K. Kim, S. Bengió, I. Yu. Sklyadneva, A. Leonardo, S. V. Eremeev, E. V. Chulkov, and Ph. Hofmann, Phys. Rev. B: Condens. Matter 75, 153404 (2007).

    Article  ADS  Google Scholar 

  37. S. V. Eremeev and E. V. Chulkov, Phys. Solid State 51(4), 854 (2009).

    Article  ADS  Google Scholar 

  38. R. Keiling, W.-D. Schöne, and W. Ekardt, Chem. Phys. Lett. 354, 376 (2002).

    Article  ADS  Google Scholar 

  39. Ph. Hofmann, I. Yu. Sklyadneva, E. D. L. Rienks, and E. V. Chulkov, New J. Phys. 11, 125005 (2009).

    Article  ADS  Google Scholar 

  40. P. Straube, F. Pforte, T. Michalke, K. Berge, A. Gerlach, and A. Goldmann, Phys. Rev. B: Condens. Matter 61, 14072 (2000).

    Article  ADS  Google Scholar 

  41. A. Mugarza, A. Mascaraque, V. Repain, S. Rousset, K. N. Altmann, F. J. Himpsel, Yu. M. Koroteev, E. V. Chulkov, F. J. García de Abajo, and J. E. Ortega, Phys. Rev. B: Condens. Matter 66, 245419 (2002).

    Article  ADS  Google Scholar 

  42. S. M. Dounce, M. Yang, and H.-L. Dai, Phys. Rev. B: Condens. Matter 67, 205410 (2003).

    Article  ADS  Google Scholar 

  43. G. A. Somorjai, in Elementary Reaction Step in Heterogeneous Catalysis, Ed. by R. W. Joyner and R. A. Van Santen (Kluwer, Dordrecht, 1993), p. 3.

    Chapter  Google Scholar 

  44. E. V. Chulkov, V. M. Silkin, and P. M. Echenique, Surf. Sci. 391, L1217 (1997); E. V. Chulkov, V. M. Silkin, and P. M. Echenique, Surf. Sci. 437, 330 (1999).

    Article  Google Scholar 

  45. S. S. Tsirkin, S. V. Eremeev, and E. V. Chulkov, Phys. Solid State (St. Petersburg) 52(1), 188 (2010).

    Article  ADS  Google Scholar 

  46. S. S. Tsirkin, S. V. Eremeev, and E. V. Chulkov, Surf. Sci. 604, 804 (2010).

    Article  ADS  Google Scholar 

  47. S. S. Tsirkin, S. V. Eremeev, and E. V. Chulkov, Phys. Rev. B: Condens. Matter 84, 115451 (2011).

    Article  ADS  Google Scholar 

  48. S. V. Eremeev, S. S. Tsirkin, and E. V. Chulkov, JETP 110(5), 788 (2010).

    Article  ADS  Google Scholar 

  49. S. V. Eremeev, S. S. Tsirkin, and E. V. Chulkov, Phys. Rev. B: Condens. Matter 82, 035424 (2010).

    Article  ADS  Google Scholar 

  50. S. V. Eremeev, S. S. Tsirkin, and E. V. Chulkov, Phys. Solid State (St. Petersburg) 52(8), 1768 (2010).

    Article  ADS  Google Scholar 

  51. S. S. Tsirkin and S. V. Eremeev, Russ. Phys. J. 54(1), 92 (2011).

    Article  MATH  Google Scholar 

  52. S. S. Tsirkin and S. V. Eremeev, Russ. Phys. J. 54(11), 1196 (2011).

    Article  Google Scholar 

  53. L. Hedin, Phys. Rev. [Sect.] A 139, 796 (1965).

    ADS  Google Scholar 

  54. F. J. Himpsel and D. E. Eastman, Phys. Rev. B: Condens. Matter 18, 5236 (1978).

    Article  ADS  Google Scholar 

  55. N. V. Smith, C. T. Chen, J. M. Tranquada, and P. D. Johnson, Phys. Rev. B: Condens. Matter 38, 12259 (1988).

    Article  ADS  Google Scholar 

  56. P. M. Echenique, J. M. Pitarke, E. V. Chulkov, and A. Rubio, Chem. Phys. 251, 1 (2000).

    Article  Google Scholar 

  57. A. Garcia-Lekue, J. M. Pitarke, E. V. Chulkov, A. Liebsch, and P. M. Echenique, Phys. Rev. B: Condens. Matter 68, 045103 (2003).

    Article  ADS  Google Scholar 

  58. J. J. Quinn and R. A. Ferrell, Phys. Rev. 112, 812 (1958).

    Article  MathSciNet  ADS  MATH  Google Scholar 

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Correspondence to S. S. Tsirkin.

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Original Russian Text © S.S. Tsirkin, S.V. Eremeev, E.V. Chulkov, 2012, published in Zhurnal Eksperimental’noi i Teoreticheskoi Fiziki, 2012, Vol. 142, No. 4, pp. 761–769.

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Tsirkin, S.S., Eremeev, S.V. & Chulkov, E.V. Lifetimes of electronic excitations in unoccupied surface states and the image potential states on Pd(110). J. Exp. Theor. Phys. 115, 673–680 (2012). https://doi.org/10.1134/S1063776112090154

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