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SIMS on the Helium Ion Microscope: A Powerful Tool for High-Resolution High-Sensitivity Nano-Analytics

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Helium Ion Microscopy

Part of the book series: NanoScience and Technology ((NANO))

Abstract

Secondary Ion Mass Spectrometry (SIMS ) is an extremely powerful technique for analysing surfaces, owing in particular to its excellent sensitivity , high dynamic range , very high mass resolution , and ability to differentiate between isotopes . The combination of He/Ne microscopy and SIMS makes it possible not only to obtain SIMS information limited only by the size of the probe–sample interaction (~10 nm), but also to directly correlate such SIMS images with high-resolution (0.5 nm) secondary electron images of the same zone taken at the same time. This chapter will discuss the feasibility of combining SIMS with Helium Ion Microscopy from a fundamental and instrumental point of view.

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References

  1. J.P. Biersack, L.G. Haggmark, Nucl. Instrum. Methods 174, 257 (1980)

    Article  ADS  Google Scholar 

  2. J.P. Biersack, W. Eckstein, Appl. Phys. A-Matter 34, 73 (1984)

    Article  ADS  Google Scholar 

  3. W. Eckstein, W. Möller, Nucl. Instrum. Methods Phys. Res. B 7(8), 727 (1985)

    Article  ADS  Google Scholar 

  4. T. Wirtz, P. Philipp, J.-N. Audinot, D. Dowsett, S. Eswara, Nanotechnology 26, 434001 (2015)

    Article  ADS  Google Scholar 

  5. W. Moller, W. Eckstein, Nucl. Instrum. Methods Phys. Res. B 230, 814 (1984)

    Article  ADS  Google Scholar 

  6. W. Eckstein, J.P. Biersack, Appl. Phys. A-Matter 37, 95 (1985)

    Article  ADS  Google Scholar 

  7. W. Moller, W. Eckstein, J.P. Biersack, Comput. Phys. Commun. 51, 355 (1988)

    Article  ADS  Google Scholar 

  8. J. Lindhard, M. Scharff, Phys. Rev. 124, 128 (1961)

    Article  ADS  Google Scholar 

  9. K. Wittmaack, Surf. Sci. Rep. 68, 108 (2013)

    Article  ADS  Google Scholar 

  10. K. Wittmaack, Anal. Chem. 86, 5962 (2014)

    Article  Google Scholar 

  11. G. Slodzian, Surf. Sci. 48, 161 (1975)

    Article  ADS  Google Scholar 

  12. G. Slodzian, Phys. Scr. T6, 54 (1983)

    Article  ADS  Google Scholar 

  13. K. Franzreb, J. Lörincik, P. Williams, Surf. Sci. 573, 291 (2004)

    Article  ADS  Google Scholar 

  14. M. Bernheim, G. Slodzian, Journal de Physique Lettres 38, L325 (1977)

    Article  Google Scholar 

  15. M. Bernheim, J. Rebière, G. Slodzian, Proceedings of the Second International Conference on Secondary Ion Mass Spectrometry (SIMS II);40 (1979)

    Google Scholar 

  16. T. Wirtz, H.N. Migeon, Surf. Sci. 557, 57 (2004)

    Article  ADS  Google Scholar 

  17. T. Wirtz, H.N. Migeon, Appl. Surf. Sci. 222, 186 (2004)

    Article  ADS  Google Scholar 

  18. P. Philipp, T. Wirtz, H.N. Migeon, H. Scherrer, Int. J. Mass Spectrom. 253, 71 (2006)

    Article  ADS  Google Scholar 

  19. P. Philipp, T. Wirtz, H.N. Migeon, H. Scherrer, Appl. Surf. Sci. 252, 7205 (2006)

    Article  ADS  Google Scholar 

  20. A. Benninghoven, Werner H. Wand, F.G. Rüdenauer, Secondary ion mass spectrometry: basic concepts, instrumental aspects, applications and trends (Wiley-Interscience, New York, Chichester, Brisbane, Toronto, Singapore, 1987)

    Google Scholar 

  21. Y. Gao, J. Appl. Phys. 64(7), 3760 (1988)

    Article  ADS  Google Scholar 

  22. T. Wirtz, H.N. Migeon, H. Scherrer, Int. J. Mass Spectrom. 225, 135 (2003)

    Article  ADS  Google Scholar 

  23. H. Gnaser, H. Oechsner, Surf. Interface Anal. 21, 257 (1994)

    Article  Google Scholar 

  24. Y. Gao, Y. Marie, F. Saldi, H.N. Migeon, Proceedings of the Ninth International Conference on Secondary Ion Mass Spectrometry (SIMS IX) 406 (1993)

    Google Scholar 

  25. W. Compston, S.W.J. Clement, Appl. Surf. Sci. 252, 7089 (2006)

    Article  ADS  Google Scholar 

  26. Y. Fleming, T. Wirtz, Beilstein J. Nanotechnol. 6, 1091 (2015)

    Article  Google Scholar 

  27. H. Oechsner, H. Schoof, E. Stumpe, Surf. Sci. 76, 343 (1978)

    Article  ADS  Google Scholar 

  28. W. Vandervorst, Appl. Surf. Sci. 255, 805 (2008)

    Article  ADS  Google Scholar 

  29. M.Y. Chan, P.S. Lee, V. Ho, H.L. Seng, J. Appl. Phys. 102 (2007)

    Google Scholar 

  30. A. Redinger, K. Hönes, X. Fontan, V. Izquierdo-Roca, E. Saucedo, N. Valle, A. Prez-Rodriguez, S. Siebentritt, Appl. Phys. Lett. 98 (2011)

    Google Scholar 

  31. T. Wirtz, N. Vanhove, L. Pillatsch, D. Dowsett, S. Sijbrandij, J. Notte, Appl. Phys. Lett. 101, 041601 (2012)

    Article  ADS  Google Scholar 

  32. J.F. Ziegler, J. Biersack, U. Pand Littmark, The Stopping and Range of Ions in Solids (Pergamon, 1985)

    Google Scholar 

  33. L. Pillatsch, N. Vanhove, D. Dowsett, S. Sijbrandij, J. Notte, T. Wirtz, Appl. Surf. Sci. 282, 908 (2013)

    Article  ADS  Google Scholar 

  34. T. Wirtz, H.N. Migeon, Appl. Surf. Sci. 231–232, 940 (2004)

    Article  Google Scholar 

  35. J. Orloff, L.W. Swanson, M. Utlaut, J. Vac. Sci. Technol. B 14(6), 3759 (1996)

    Article  Google Scholar 

  36. V. Castaldo, C.W. Hagen, P. Kruit, E. van Veldhoven, D. Maas, J. Vac. Sci. Technol. B 27, 3196 (2009)

    Article  Google Scholar 

  37. M. Guilhaus, D. Selby, V. Mlynski, Mass Spectrom. Rev. 19, 65 (2005)

    Article  Google Scholar 

  38. D. Dowsett, T. Wirtz, N. Vanhove, L. Pillatsch, S. Sijbrandij, J. Notte, J. Vac. Sci. Technol. B 30, 06F602 (2012)

    Article  Google Scholar 

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Acknowledgments

Some of the work presented in this paper was funded by the National Research Fund of Luxembourg by the grants FNR-MAT-08-01, C09/MS/13, C10/MS/801311 and C13/MS/5951975.

This work was supported in part by the Intelligence Advanced Research Projects Activity (IARPA) via Air Force Research Laboratory (AFRL) contract number FA8650-11-C-7100. The U.S. government is authorised to reproduce and distribute reprints for governmental purposes, notwithstanding any copyright annotation thereon. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing the official policies or endorsements, either expressed or implied, of IARPA, AFRL, or the U.S. government.

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Correspondence to Tom Wirtz .

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Wirtz, T., Dowsett, D., Philipp, P. (2016). SIMS on the Helium Ion Microscope: A Powerful Tool for High-Resolution High-Sensitivity Nano-Analytics. In: Hlawacek, G., Gölzhäuser, A. (eds) Helium Ion Microscopy. NanoScience and Technology. Springer, Cham. https://doi.org/10.1007/978-3-319-41990-9_13

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