Abstract
Second Harmonic Generation (SHG) at a metallic surface was first reported by F. Brown et al. [1] in 1965. At the same time, Jha [2] established that this phenomenon is a surface effect. Indeed, in bulk centrosymmetric media, even order nonlinear (NL) effects, in particular SHG, are forbidden. However, there is, by geometry, a break of the symmetry at the surface. The second harmonic (SH) signal is generated because of the discontinuities occurring at the surface. A second source term is due to the decay of the pump field in the medium. These initial ideas are well described in a famous paper by Bloembergen et al. [3] published in 1968.
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Coutaz, JL. (1990). Surface Enhanced Second Harmonic Generation from Metals. In: Keller, O. (eds) Nonlinear Optics in Solids. Springer Series on Wave Phenomena, vol 9. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-84206-1_5
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DOI: https://doi.org/10.1007/978-3-642-84206-1_5
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