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Iron(III) Spin Crossover Compounds

  • Chapter
Spin Crossover in Transition Metal Compounds I

Part of the book series: Topics in Current Chemistry ((TOPCURRCHEM,volume 233))

Abstract

In this chapter, selected results obtained so far on Fe(III) spin crossover compounds are summarized and discussed. Fe(III) spin transition materials of ligands containing chalcogen donor atoms are considered with emphasis on those of N,N-disubstituted-dithiocarbamates, N,N-disubstituted-XY-carbamates (XY=SO, SSe, SeSe), X-xanthates (X=O, S), monothio-β-diketonates and X-semicarbazones (X=S, Se). In addition, attention is directed to Fe(III) spin crossover systems of multidentate Schiff base-type ligands. Examples of spin inter-conversion in Fe(III) compounds induced by light irradiation are given.

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Abbreviations

H2thsa:

Salicylaldehyde thiosemicarbazone

H2Phthsa:

Salicylaldehyde phenylthiosemicarbazone

H2sesa:

Salicylaldehyde selenosemicarbazone

H2thpu:

Pyruvic acid thiosemicarbazone

H2sespu:

Pyruvic acid selenosemicarbazone

H2thpy:

Pyridoxal 4-R-thiosemicarbazone

H-3-OEt-salAPA:

Schiff base derived from 3-ethoxysalicylaldehyde and N-aminopropylaziridine

HsalAEA:

Schiff base derived from salicylaldehyde and N-(2-aminoethyl)aziridine

Hsapa:

N-Salicylidene-2-pyridylmethylamine

Hvapa:

N-(3-Methoxysalicylidene)-2-pyridylmethylamine

H-3-CH3OSPH:

Schiff base derived from 3-methoxysalicylaldehyde and 2-pyridylhydrazine

H-X-salmeen:

Schiff base derived from X-salicylaldehyde and N-methylethylenediamine

H-X-saleen:

Schiff base derived from X-salicylaldehyde and N-ethylethylenediamine

H-X-salbzen:

Schiff base derived from N-benzylethylenediamine and X-substituted salicylaldehyde

Hacea:

Schiff base derived from 2,4-pentanedione and 1,2-diaminoethane

Hacpa:

N-(1-Acetyl-2-propylidene)(2-pyridylmethyl)amine

Hbzpa:

(1-Benzoylpropen-2-yl)(2-pyridylmethyl)amine

Hqsal:

N-(8-Quinolyl)-salicylaldimine

Hpap:

2-Hydroxyphenyl-(2-pyridyl)-methaneimine

cyclam:

1,4,8,11-Tetraazacyclotetradecane

tcyclam:

1,4,8,11-Tetramethyl-1,4,8,11-tetraazacyclotetradecane

H2amben:

Schiff base derived from 2-aminobenzaldehyde and ethylenediamine

H2salen:

N,N′-Ethylenebis(salicylideneamine)

H2salphen:

N,N′-o-Phenylenebis(salicylideneamine)

Him:

Imidazole

H2-3-OCH3-salpen:

N,N′-1,2-Propylenebis(3-methoxysalicylideneamine)

H2-3-OC2H5-sal-CH3-phen:

N,N′-3,4-Toluenebis(3-ethoxysalicylideneamine)

H2acen:

N,N′-Ethylenebis(acetylacetonylideneamine)

H2bzacen:

N,N′-Ethylenebis(benzoylacetonylideneamine)

H2salacen:

Ethylene(N-acetylacetonylideneimine)(N′-α-methylsalicylideneimine)

H2salten:

N,N′-Bis([2-hydroxy-phenyl)methylene]-4-azaheptane-1,7-diamine

H2bpN:

N,N′-Bis([2-hydroxy-phenyl)phenylmethylene]-4-azaheptane-1,7-diamine

H2mbpN:

N,N′-Bis([2-hydroxy-5-methyl-phenyl)phenylmethylene]-4-azaheptane-1,7-diamine

H2sal2trien:

Schiff base obtained from the 1:2 condensation of triethylenetetramine with salicylaldehyde

H2acac2trien:

Schiff base obtained from the 1:2 condensation of triethylenetetramine with acetylacetone

H2bzac2trien:

Schiff base obtained from the 1:2 condensation of triethylenetetramine with benzoylacetone

H2tfac2trien:

Schiff base obtained from the 1:2 condensation of triethylenetetramine with trifluoroacetylacetone

Mepepy:

1-(Pyridin-4-yl)-2-(N-methylpyrrol-2-yl)-ethene

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Acknowledgement

P.J.v.K. gratefully acknowledges the kind provision of work facilities at the Johannes-Gutenberg-University by Professor Philipp Görlich.

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Authors and Affiliations

  1. Stratingh Institute for Chemistry and Chemical Engineering, University of Groningen, Nijenborgh 4, 9747 AG, Groningen, The Netherlands

    Petra J. van Koningsbruggen

  2. Department of Chemistry, Kyushu University, 6-10-1 Hakozaki, Higashi-ku, Fukuoka 812-8581, Japan

    Yonezo Maeda

  3. Department of Chemistry, University of Tsukuba, Tennodai 1-1-1, Tsukuba 305-8571, Japan

    Hiroki Oshio

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  1. Petra J. van Koningsbruggen
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  2. Yonezo Maeda
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  3. Hiroki Oshio
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Correspondence to Petra J. van Koningsbruggen .

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P. Gütlich H.A. Goodwin

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van Koningsbruggen, P.J., Maeda, Y., Oshio, H. Iron(III) Spin Crossover Compounds. In: Gütlich, P., Goodwin, H. (eds) Spin Crossover in Transition Metal Compounds I. Topics in Current Chemistry, vol 233. Springer, Berlin, Heidelberg. https://doi.org/10.1007/b95409

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  • DOI: https://doi.org/10.1007/b95409

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